The purpose of this study is to propose and compare methods for measuring individual spray cone angles using spray cross-section images. In direct injection gasoline engines, it was believed that the distribution of air-fuel mixture in the combustion chamber directly affected combustion performance and emission formation. However, since gasoline direct injection (GDI) injectors have a small injection angle, interference between individual spray plumes occurs. Therefore, GDI injectors have only measured the spray angle of the entire spray. To overcome these limitations, three methods of indirectly measuring the spray cone angles of individual spray plume were presented and compared by forming sheet beams using Nd:YAG laser and acquiring spray cross-section images. Each method currently has advantages and disadvantages, and research to apply the method suitable for various GDI injectors needs to be continued.